That's a better set overall I'd say. The SNES games have a bit more bang for your buck compared to the NES games as their gameplay still holds up even today, they have more length to them so you'll be attached to them for longer, and with the potential aforementioned online multiplayer you could be able to play with friends on top of that. It's still not ideal as the majority of these have been rereleased multiple times before (offhand, I think only a couple like Star Fox 2 and Demon's Crest have been limited in that regard), but at least there's more offered here to get you invested.
For me personally, Yoshi's Island, Star Fox 2, and Breath of Fire 2 are games I've been wanting to play so that's good for me. I also love Super Metroid and Demon's Crest, so I wouldn't mind replaying those two again.