My Fav moments have to be;
Riding the Train in ST (and music was so catchy!)
Beating ST (first ever Zelda game complete)
Pulling the Master Sword out in Oot (that music then the plot twist)
Fighting Ganondorf in a tennis match
Ganon. Nuff said.
Using the Wall Ability in ALBW (it was a really fun mechanic imo)
Classic Link gameplay (it's actually very fun)
The Final Boss in ALBW (man it was hard)
Using the Motion Control on SS (am I the only one who enjoyed?)
Meeting Fi for the first time and that music (oh many)
Fighting Ghriham (every battle)
Flying on a Loftwing
Getting the Master Sword.
Zelda (she had so much character)
Zelda x Link that is implied.
The final scene with Fi (I am willing to admit I bursted into tears)
MM in it's entirety. I literally can not choose a single point, I loved the whole thing. the characters, the mechanics, the music, the fights, it was all amazing. It is my fav Zelda of them all and has my Fav Link of all time as the main character.